TY - JOUR
T1 - Multifunctional Hydrothermal-Carbonized Sugarcane for Highly Efficient Direct Solar Steam Generation
AU - Wei, Anyun
AU - Cui, Kewen
AU - Wang, Pengfei
AU - Gu, Yufei
AU - Wang, Xiaoyang
AU - Mu, Xiaojiang
AU - Tian, Yongzhi
AU - Zhou, Jianhua
AU - Sun, Zhiqiang
AU - Chen, Yulian
AU - Zhang, Jiahong
AU - Liu, Jing
AU - Miao, Lei
N1 - Funding Information:
This work was supported by National Key Research and Development Program of China (grant no. 2017YFE0198000), Natural Science Foundation of Guangxi Province (grant nos. 2019GXNSFFA245010, 2019GXNSFAA245042, and 2019GXNSFBA245028), Scientific Research and Technology Development Program of Guangxi (grant nos. AD18281057, AD19110072, AD19245177, and AD19245160), and the Basic Ability Promotion Project for Young College Teachers in Guangxi Zhuang Autonomous Region (grant no. 2018KY020).
Funding Information:
This work was supported by National Key Research and Development Program of China (grant no. 2017YFE0198000), Natural Science Foundation of Guangxi Province (grant nos. 2019GXNSFFA245010, 2019GXNSFAA245042, and 2019GXNSFBA245028), Scientific Research and Technology Development Program of Guangxi (grant nos. AD18281057, AD19110072, AD19245177, and AD19245160), and the Basic Ability Promotion Project for Young College Teachers in Guangxi Zhuang Autonomous Region (grant no. 2018KY020).
Publisher Copyright:
© 2021 Wiley-VCH GmbH
PY - 2021/3
Y1 - 2021/3
N2 - Solar steam generation is an environmentally friendly water treatment method that produces clean water using solar energy. However, it is still a challenge to effectively prevent the performance deterioration when most photothermal conversion materials are used to evaporate high-concentration salt-containing wastewater or strong acid/alkali solution. Herein, a stable and effective solar evaporator is designed using natural sugarcane, where sucrose is simply dehydrated into carbon particles by hydrothermal reaction in sulfuric acid. With a honeycomb structure, it not only enables water transport capacity but also promotes sunlight absorption. Sulfuric acid hydrothermal carbonized sugarcane (SHCSC) can reach up to 95.36% solar absorption in a wide wavelength range (200–2500 nm) and a high evaporation rate of 2.32 kg m−2 h−1 under 1 sun illumination. More importantly, SHCSC has an excellent adsorption capacity with ion removal rate of 99.9% even under artificial wastewater containing 1000 mg L−1 of mixed metal ions. SHCSC also can perform efficiently and stably at a high evaporation rate above 2.2 kg m−2 h−1 in strong acidic or alkaline wastewater. These findings suggest that SHCSC can be potentially applied to the efficient harvest of clean water from the high-concentration wastewater containing acid, alkali, and mixed metal ions.
AB - Solar steam generation is an environmentally friendly water treatment method that produces clean water using solar energy. However, it is still a challenge to effectively prevent the performance deterioration when most photothermal conversion materials are used to evaporate high-concentration salt-containing wastewater or strong acid/alkali solution. Herein, a stable and effective solar evaporator is designed using natural sugarcane, where sucrose is simply dehydrated into carbon particles by hydrothermal reaction in sulfuric acid. With a honeycomb structure, it not only enables water transport capacity but also promotes sunlight absorption. Sulfuric acid hydrothermal carbonized sugarcane (SHCSC) can reach up to 95.36% solar absorption in a wide wavelength range (200–2500 nm) and a high evaporation rate of 2.32 kg m−2 h−1 under 1 sun illumination. More importantly, SHCSC has an excellent adsorption capacity with ion removal rate of 99.9% even under artificial wastewater containing 1000 mg L−1 of mixed metal ions. SHCSC also can perform efficiently and stably at a high evaporation rate above 2.2 kg m−2 h−1 in strong acidic or alkaline wastewater. These findings suggest that SHCSC can be potentially applied to the efficient harvest of clean water from the high-concentration wastewater containing acid, alkali, and mixed metal ions.
KW - desalination
KW - high-concentration wastewater
KW - hydrothermal carbonized sugarcane
KW - solar steam generation
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U2 - 10.1002/solr.202000782
DO - 10.1002/solr.202000782
M3 - Article
AN - SCOPUS:85100198805
SN - 2367-198X
VL - 5
JO - Solar RRL
JF - Solar RRL
IS - 3
M1 - 2000782
ER -