TY - JOUR
T1 - Recent progress of carbon-based electrocatalytic materials in Lithium-based batteries
AU - Wang, Pengfei
AU - Zhang, Jiahong
AU - Peng, Ying
AU - Hu, Xiulan
AU - Miao, Lei
AU - Ishizaki, Takahiro
N1 - Funding Information:
The authors would like to acknowledge for the financial support, Grant-in-Aid for Scientific Research (B) (No. 19H02482 ), start-up (No. 20K22486 ) and Challenging Research (Exploratory) (No. 21K18835 ) from Japan Society for the Promotion of Science , Japan Science and Technology Agency (JST) under Program on Open Innovation Platform with Enterprises, Research Institute and Academia (OPERA) (No. 18072116 ), and JST , Strategic International Collaborative Research Program (SICORP) (No. JPMJSC18H1 ).
Funding Information:
The authors would like to acknowledge for the financial support, Grant-in-Aid for Scientific Research (B) (No. 19H02482), start-up (No. 20K22486) and Challenging Research (Exploratory) (No. 21K18835) from Japan Society for the Promotion of Science, Japan Science and Technology Agency (JST) under Program on Open Innovation Platform with Enterprises, Research Institute and Academia (OPERA) (No. 18072116), and JST, Strategic International Collaborative Research Program (SICORP) (No. JPMJSC18H1).
Publisher Copyright:
© 2022 Elsevier B.V.
PY - 2022/7
Y1 - 2022/7
N2 - Lithium‑oxygen, −air, -CO2 are three typical types of Lithium-based batteries, which offer a promising, sustainable, and environment-friendly solution to construct carbon neutral society. Carbon-based cathodes provide active sites for mass and electronic transfer among Li, Li+, O2, Li2O2, LiO2. The synthesis methods of carbon cathode can affect the performance of Lithium-based battery. This review summarizes the fundamentals of carbon-based oxygen evolution reaction (OER) and oxygen reduced reaction (ORR) electrocatalytic reactions, and then explore a few key concerns on the interrelation between synthesis methods and electrocatalytic activities. Then, the most important tactics: defect engineering, heteroatom doping, and structure optimization for enhancement of electrocatalytic activity are presented. Finally, the most recent advances of carbon-based materials from dimensional views are also discussed. The review would provide insightful opportunities as well as the current challenges to accelerate the research and application on carbon-based materials for Lithium-based batteries.
AB - Lithium‑oxygen, −air, -CO2 are three typical types of Lithium-based batteries, which offer a promising, sustainable, and environment-friendly solution to construct carbon neutral society. Carbon-based cathodes provide active sites for mass and electronic transfer among Li, Li+, O2, Li2O2, LiO2. The synthesis methods of carbon cathode can affect the performance of Lithium-based battery. This review summarizes the fundamentals of carbon-based oxygen evolution reaction (OER) and oxygen reduced reaction (ORR) electrocatalytic reactions, and then explore a few key concerns on the interrelation between synthesis methods and electrocatalytic activities. Then, the most important tactics: defect engineering, heteroatom doping, and structure optimization for enhancement of electrocatalytic activity are presented. Finally, the most recent advances of carbon-based materials from dimensional views are also discussed. The review would provide insightful opportunities as well as the current challenges to accelerate the research and application on carbon-based materials for Lithium-based batteries.
KW - Carbon materials
KW - Electrocatalysts
KW - Lithium-based batteries
KW - OER/ORR
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U2 - 10.1016/j.susmat.2021.e00384
DO - 10.1016/j.susmat.2021.e00384
M3 - Review article
AN - SCOPUS:85123121328
SN - 2214-9937
VL - 32
JO - Sustainable Materials and Technologies
JF - Sustainable Materials and Technologies
M1 - e00384
ER -